ISSN 1009-6248CN 61-1149/P 双月刊

主管单位:中国地质调查局

主办单位:中国地质调查局西安地质调查中心
中国地质学会

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    浅层地下水硝酸盐来源解析及健康风险评价:以渭南市华州区为例

    Identification of Nitrate Sources and Main Controlling Factors in Shallow Groundwater Based on MixSIAR and Random Forest Model

    • 摘要: 作为全球水资源中最普遍的污染物,NO3−主控因素和来源的识别对NO3−污染控制至关重要。本研究基于人体健康风险、随机森林模型、同位素和MixSIAR模型等方法,分析了华州区浅层地下水NO3−分布特征和潜在风险,揭示了浅层地下水NO3−的重要因素和主要来源。结果表明:华州区浅层地下水NO3−浓度呈西高东低趋势分布,西南部尤为显著,NO3−浓度高达271mg/L。主要控制NO3−浓度的指标依次为:EC>ORP>Ca2+>Mg2+>T>TDS>HCO3−。NO3−来源以土壤氮和粪肥及污水为主,且粪便及污水对NO3−含量贡献率最大(63.8%),其次是土壤氮(19%)和化肥(12.7%)。长期饮用研究区NO3−浓度较高的浅层地下水对人类健康具有潜在风险,特别是儿童,其HHRA评估风险值高达7.904。

       

      Abstract: As the most common pollutant in global water resources, the identification of the main controlling factors and sources of NO3− is crucial to the control of NO3− pollution. Based on methods such as human health risk model, random forest model, isotope and MixSIAR model, this study analyzed the distribution characteristics and potential risks of shallow groundwater NO3− in Huazhou District, and revealed the main controlling factors and main sources of shallow groundwater NO3−. The results show that the shallow groundwater NO3− concentration in Huazhou District is high in the west and low in the east, especially in the southwest. The NO3− concentration is as high as 271 mg/L. The main factors controlling NO3− concentration being EC>ORP>Ca2+>Mg2+>T>TDS>HCO3−. The main sources of NO3− are soil nitrogen and manure & sewage. The manure & sewage contributes the most to the NO3− content (63.8%), followed by soil nitrogen (19%) and chemical fertilizer (12.7%). Long-term drinking of shallow groundwater with high NO3− concentration in the study area has potential risks to human health, especially for children, whose HHRA assessment risk is as high as 7.904.

       

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