ISSN 1009-6248CN 61-1149/P 双月刊

主管单位:中国地质调查局

主办单位:中国地质调查局西安地质调查中心
中国地质学会

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    浅层地下水硝酸盐来源解析及健康风险评价:以渭南市华州区为例

    Identification of Nitrate Sources and Main Controlling Factors in Shallow Groundwater Based on MixSIAR and Random Forest Model

    • 摘要: 作为全球水资源中最普遍的污染物,NO3主控因素和来源的识别对NO3污染控制至关重要。本研究基于人体健康风险、随机森林模型、同位素和MixSIAR模型等方法,分析了华州区浅层地下水NO3分布特征和潜在风险,揭示了浅层地下水NO3的重要因素和主要来源。结果表明:华州区浅层地下水NO3浓度呈西高东低趋势分布,西南部尤为显著,NO3浓度高达271mg/L。主要控制NO3浓度的指标依次为:EC>ORP>Ca2+>Mg2+>T>TDS>HCO3。NO3来源以土壤氮和粪肥及污水为主,且粪便及污水对NO3含量贡献率最大(63.8%),其次是土壤氮(19%)和化肥(12.7%)。长期饮用研究区NO3浓度较高的浅层地下水对人类健康具有潜在风险,特别是儿童,其HHRA评估风险值高达7.904。

       

      Abstract: As the most common pollutant in global water resources, the identification of the main controlling factors and sources of NO3 is crucial to the control of NO3 pollution. Based on methods such as human health risk model, random forest model, isotope and MixSIAR model, this study analyzed the distribution characteristics and potential risks of shallow groundwater NO3 in Huazhou District, and revealed the main controlling factors and main sources of shallow groundwater NO3. The results show that the shallow groundwater NO3 concentration in Huazhou District is high in the west and low in the east, especially in the southwest. The NO3 concentration is as high as 271 mg/L. The main factors controlling NO3 concentration being EC>ORP>Ca2+>Mg2+>T>TDS>HCO3. The main sources of NO3 are soil nitrogen and manure & sewage. The manure & sewage contributes the most to the NO3 content (63.8%), followed by soil nitrogen (19%) and chemical fertilizer (12.7%). Long-term drinking of shallow groundwater with high NO3 concentration in the study area has potential risks to human health, especially for children, whose HHRA assessment risk is as high as 7.904.

       

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